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By Massimo Baroncini

This thesis makes a speciality of the bottom-up layout, building and operation of supramolecular platforms able to behaving as units and machines at the molecular scale, that is a subject matter of significant curiosity in nanoscience and a desirable problem in nanotechnology. specifically, the platforms investigated right here contain: polyviologen dendrimers able to behaving as hosts and chargestoring units; molecular machines in keeping with pseudorotaxanes/rotaxanes and operated through photoinduced proton move, or photoisomerization reactions; and a straightforward unimolecular multiplexer/demultiplexer. The structures were characterised utilizing numerous ideas together with absorption and emission spectra, laser flash photolysis, NMR spectroscopy, electrochemical experiments, stopped move measurements. This learn addresses plenty of open difficulties within the nanosciences, facing a variety of the main complex purposes of supramolecular systems.

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